CHINESE JOURNAL OF ENERGETIC MATERIALS
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基于1,2,3-三唑骨架的含能化合物研究进展
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1.南京理工大学化学与化工学院, 江苏 南京 210094;2.北京航天试验技术研究所, 航天绿色推进剂研究与应用北京市重点实验室, 北京 100074

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Research Progress of Energetic Compounds based on 1,2,3-Triazole Frameworks
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1.School of Chemistry and Chemical Engineering,Nanjing University of Science and Technology,Nanjing 210094,China;2.Beijing Institute of Aerospace Testing Technology,Beijing Key Laboratory of Research and Application for Arospace Green Propellants, Beijing 100074,China

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    摘要:

    本文综述了自20世纪60年代以来构建1,2,3-三唑类含能材料的4种主要方式以及相应的研究进展,包括:1)基于1-氨基-1,2,3-三唑构建的含能化合物;2)基于二氰基1,2,3-三唑构建的含能化合物;3)叠氮参与环合反应制备1,2,3-三唑类含能化合物;4)1,2,3-三唑参与构建的稠环类含能化合物。通过对具有代表性的1,2,3-三唑含能化合物的分子结构以及相应的理化特性进行分析,深层次地理解含能材料的结构对其能量水平以及稳定性的影响。同时,对性能突出的1,2,3-三唑含能化合物的潜在应用价值进行了展望,为设计和开发下一代高能量密度材料提供参考。

    Abstract:

    This review focused on the four major construction methods of 1,2,3-triazole energetic materials and corresponding research progress since the 1960s, including: Ⅰ) energetic compounds constructed based on 1-amino-1,2,3-triazole; Ⅱ) energetic compounds constructed based on dicyano substituted 1,2,3-triazole; Ⅲ) 1,2,3-triazole based energetic compounds prepared through azide involved cyclization reaction; Ⅳ) fused polycyclic energetic compounds built from 1,2,3-triazole. By analyzing the relationship between the molecular structure and energetic properties of several representative 1,2,3-triazole based energetic compounds, the influence of molecular structures on their energetic performances and stabilities could be profoundly clarified. Meanwhile, the potential application values of the mentioned high-performance 1,2,3-triazole based energetic compounds, such as their application prospects of main explosives, heat-resistant explosives and lead-free primary explosive, were discussed, providing a reference for the design and development of next-generation high energy density materials (HEDMs).

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引用本文

蔺向阳,曹宇鹏,张西亚.基于1,2,3-三唑骨架的含能化合物研究进展[J].含能材料, 2023, 31(1):92-106. DOI:10.11943/CJEM2022008.
LIN Xiang-yang, CAO Yu-peng, ZHANG Xi-ya. Research Progress of Energetic Compounds based on 1,2,3-Triazole Frameworks[J]. Chinese Journal of Energetic Materials, 2023, 31(1):92-106. DOI:10.11943/CJEM2022008.

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历史
  • 收稿日期: 2022-01-09
  • 最后修改日期: 2022-10-28
  • 录用日期: 2022-05-18
  • 在线发布日期: 2022-10-25
  • 出版日期: 2023-01-25